Crystal structural observation of C-4V-symmetric tetrathiahemicarceplexes and their equilibria

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초록

The crystal structures of tetrathiahemicarceplexes 1,4-diiodobenzene@1 and 4-iodotoluene@1 are reported. From the crystal structures and H-1 NMR experiment the kinetic versus thermodynamic complexation shifts of 4-iodotoluene@1 were observed. The four thia groups of tetrathiahemicarceplex cooperatively built the bottleneck' leading to the equilibrium shift of carceroisomers. (C) 2011 Elsevier Ltd. All rights reserved.

키워드

CarceroisomerOrientational isomerTetrathiahemicarceplexBottleneck effectASSEMBLING HETERODIMERIC CAPSULEORIENTATIONAL ISOMERISMHYDROGEN-BONDSANION-BINDINGCARCEPLEXES
제목
Crystal structural observation of C-4V-symmetric tetrathiahemicarceplexes and their equilibria
저자
Kim, In-KyuKim, JaheonPaek, Kyungsoo
DOI
10.1016/j.tetlet.2011.09.007
발행일
2011-11-09
유형
Article
저널명
Tetrahedron Letters
52
45
페이지
6011 ~ 6014